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A Silver-Catalyzed Modular Intermolecular Access to 6,6-Spiroketals
Journal article   Open access  Peer reviewed

A Silver-Catalyzed Modular Intermolecular Access to 6,6-Spiroketals

Alexander Ahrens, Niklas F. Heinrich, Simon R. Kohl, Martha Hokamp, Matthias Rudolph, Frank Rominger and A. Stephen K. Hashmi
Advanced synthesis & catalysis, Vol.361(24), pp.5605-5615
17/12/2019

Abstract

Chemistry Chemistry, Applied Chemistry, Organic Physical Sciences Science & Technology
A modular synthesis of 6,6-spiroketals via silver catalysis is reported. By combining an intermolecular Michael addition and a 6-endo-dig cyclization, this cascade reaction allows the modular preparation of highly substituted 6,6-spiroketals by combining two substrate molecules. Established methods accessing this interesting substructure are complemented by this new transformation. The protocol tolerates diverse substitution patterns and functional groups.
url
https://doi.org/10.1002/adsc.201900988View
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