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An Ammonia-Triggered Stereocontrolled Conversion of alpha gamma-Lactone to the Central Tetrahydropyran of Pederin, Psymberin, and Onnamides D-F
Journal article   Peer reviewed

An Ammonia-Triggered Stereocontrolled Conversion of alpha gamma-Lactone to the Central Tetrahydropyran of Pederin, Psymberin, and Onnamides D-F

William J. Buffham, Nigel A. Swain, Sarah L. Kostiuk, Theo P. Goncalves and David C. Harrowven
European journal of organic chemistry, Vol.2012(6), pp.1217-1222
01/02/2012

Abstract

Chemistry Chemistry, Organic Physical Sciences Science & Technology
The onnamides, pederin, and psymberin have each attracted attention because of their potent biological activity and interesting structural features. A short (eight steps) and efficient stereocontrolled route to the central tetrahydropyran ring in these natural products has been developed from (S)-malic acid. The key sequence involves the conversion of a ?-lactone to a tetrahydropyran structure triggered by the addition of ammonia.

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