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Bronsted Base Assisted Photoredox Catalysis: Proton Coupled Electron Transfer for Remote C-C Bond Formation via Amidyl Radicals
Journal article   Peer reviewed

Bronsted Base Assisted Photoredox Catalysis: Proton Coupled Electron Transfer for Remote C-C Bond Formation via Amidyl Radicals

Jiaqi Jia, Yee Ann Ho, Raoul F. Buelow and Magnus Rueping
Chemistry : a European journal, Vol.24(53), pp.14054-14058
20/09/2018
PMID: 29939456

Abstract

Chemistry Chemistry, Multidisciplinary Physical Sciences Science & Technology
The synthesis of alkyne- and alkene-decorated lactams has been achieved through a photoredox-initiated radical cascade reaction. The developed Bronsted base assisted, photoredox-catalyzed, intramolecular 5-exo-trig cyclization/intermolecular radical addition/elimination reaction provides facile access to functionalized gamma-lactams, with good functional group tolerance and high yields.

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