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Dehydrogenative and Redox-Neutral N‑Heterocyclization of Aminoalcohols Catalyzed by Manganese Pincer Complexes
Journal article   Peer reviewed

Dehydrogenative and Redox-Neutral N‑Heterocyclization of Aminoalcohols Catalyzed by Manganese Pincer Complexes

Viktoriia Zubar, Aleksandra Brzozowska, Jan Sklyaruk and Magnus Rueping
Organometallics, Vol.41(14), pp.1743-1747
25/07/2022

Abstract

A new manganese catalyzed heterocyclization of aminoalcohols has been accomplished. A wide range of heterocycles were synthesized, including 1,2,3,4-tetrahydroquinolines, dihydroquinolinones, and 2,3,4,5-tetrahydro-1H-benzo­[b]­azepines. The reaction is performed under mild reaction conditions using air and moisture stable manganese catalysts. The desired heterocycles were obtained in good to excellent yields.

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