Abstract
We report the electronic band structure, and transport properties of the Heusler compound Co
2CrAl. The band structure calculation shows that Co
2CrAl is a true half-metallic ferromagnet with a magnetic moment of 3
μ
B per formula, characterized by a full indirect band gap of 0.475
eV at around the Fermi level in the minority-spin band. The electronic resistivity shows a power-law
T
3.15 temperature dependence at low temperatures ascribed to the unconventional one-magnon scattering processes. A negative MR maximum of –0.33% is obtained for Co
2CrAl at 300
K.