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N-Heterocyclic Carbene-Catalyzed Vinylogous Mukaiyama Aldol Reaction of -Keto Esters and -Trifluoromethyl Ketones
Journal article   Peer reviewed

N-Heterocyclic Carbene-Catalyzed Vinylogous Mukaiyama Aldol Reaction of -Keto Esters and -Trifluoromethyl Ketones

Ying Wang, Fen Xing, Mei Xue, Guang-Fen Du, Xu-Hong Guo, Kuo-Wei Huang and Bin Dai
Synthesis (Stuttgart), Vol.48(1), pp.79-84
01/01/2016

Abstract

Chemistry Chemistry, Organic Physical Sciences Science & Technology
N-Heterocyclic carbene (NHC)-catalyzed vinylogous Mukaiyama aldol reaction of ketones was developed. Under the catalysis of 5 mol% NHC, -keto esters and -trifluoromethyl ketones reacted with 2-(trimethysilyloxy)furan efficiently to produce -substituted butenolides containing adjacent quaternary and tertiary carbon centers in high yields with good diastereoselectivities.

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