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Role of the ancillary ligand in controlling the lysozyme affinity and electronic properties of terpyridine fac-Re(CO)(3) complexes
Journal article   Peer reviewed

Role of the ancillary ligand in controlling the lysozyme affinity and electronic properties of terpyridine fac-Re(CO)(3) complexes

Ahmed M. Mansour, Krzysztof Radacki and Ola R. Shehab
Dalton transactions : an international journal of inorganic chemistry, Vol.50(4), pp.1197-1201
07/02/2021
PMID: 33475110

Abstract

Chemistry Chemistry, Inorganic & Nuclear Physical Sciences Science & Technology
The lysozyme binding affinity and the electronic properties of [ReX (CO)(3)(terpy-kappa N-2(1),N-2)] (X = Br- and triazolate(COOCH2CH3,CF3)) were reported. The triazolate complex was prepared in a [3 + 2] cyclo-addition click reaction. The bromo compound reacted with lysozyme affording adducts with Re(CO)(3)(+) fragments, while the triazolate compound persisted. A red shift of the MLCT band of the triazolate compound in progressively less polar solvents may be due to the negative solvatochromism.

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