Abstract
The present research concerns the synthesis of a mesoporous composite characterized with high surface area and superior adsorption capacity in order to investigate its efficacity in removing hazardous and harmful dyes molecules from water. The synthesized mesoporous composite, MgO/g-C3N4 (MGCN), was successfully prepared through the sonication method in a methanolic solution followed by an evaporation and a calcination process. The configuration, crystalline phase, surface properties, chemical bonding, and morphological study of the fabricated nanomaterials were investigated via XRD, BET, FESEM, HRTEM, XPS, and FTIR instrumentation. The obtained nanomaterials were used as sorbents of Congo Red (CR) and Basic Fuchsin (BF) dyes from aqueous solutions. Batch elimination experimental studies reveal that the elimination of CR and BF dyes from an aqueous solution onto the MGCN surface was pH-dependent. The highest removal of CR and BF pollutants occurs, respectively, at pH 5 and 7. The absorptive elimination of CR and BF dyes into the MGCN surface was well-fitted with a pseudo-second-order kinetics and Langmuir model. In this concern, the maximum nanocomposite elimination capacity for CR and BF was observed to be 1250 and 1791 mg g−1, respectively. This investigation confirms that MGCN composite is an obvious and efficient adsorbent of CR, BF, and other organic dyes from wastewater.
•MgO/g-C3N4 Mesoporous was successfully synthesized by the sonication method.•The obtained MgO/g-C3N4 has shown interesting properties such as a high surface area. .•The obtained mesoporous were used for the removal of both Congo Red and Basic Fuchsin. .•An efficient removal for both dyes has been recorded by this mesoporous.