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TiO2 Nanotubes: Nitrogen-Ion Implantation at Low Dose Provides Noble-Metal-Free Photocatalytic H-2-Evolution Activity
Journal article   Peer reviewed

TiO2 Nanotubes: Nitrogen-Ion Implantation at Low Dose Provides Noble-Metal-Free Photocatalytic H-2-Evolution Activity

Xuemei Zhou, Volker Haeublein, Ning Liu, Nhat Truong Nguyen, Eva M. Zolnhofer, Hiroaki Tsuchiya, Manuela S. Killian, Karsten Meyer, Lothar Frey and Patrik Schmuki
Angewandte Chemie (International ed.), Vol.55(11), pp.3763-3767
07/03/2016
PMID: 26879340

Abstract

Chemistry Chemistry, Multidisciplinary Physical Sciences Science & Technology
Low-dose nitrogen implantation induces an ion and damage profile in TiO2 nanotubes that leads to co-catalytic activity for photocatalytic H-2-evolution (without the use of any noble metal). Ion implantation with adequate parameters creates this active zone limited to the top part of the tubes. The coupling of this top layer and the underlying non-implanted part of the nanotubes additionally contributes to an efficient carrier separation and thus to a significantly enhanced H-2 generation.

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